Glasslike two-level systems in minimally disordered mixed crystals

J. P. Wrubel, B. E. Hubbard, N. I. Agladze, A. J. Sievers, P. P. Fedorov, D. I. Klimenchenko, A. I. Ryskin, J. A. Campbell

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Abstract

THz spectroscopy is used to identify a broad distribution of two-level systems, characteristic of glasses, in the substitutional monatomic mixed crystal systems, Ba1-xCaxF2 and Pb1-xCaxF2. In these minimally disordered systems, two-level behavior, which was not previously known to occur, begins at a specific CaF2 concentration. The concentration dependence, successfully modeled using the statistics of the impurity distribution in the lattice, points to a collective dopant tunneling mechanism.

Original languageEnglish (US)
Article number235503
JournalPhysical Review Letters
Volume96
Issue number23
DOIs
StatePublished - Jun 23 2006
Externally publishedYes

All Science Journal Classification (ASJC) codes

  • Physics and Astronomy(all)

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    Wrubel, J. P., Hubbard, B. E., Agladze, N. I., Sievers, A. J., Fedorov, P. P., Klimenchenko, D. I., Ryskin, A. I., & Campbell, J. A. (2006). Glasslike two-level systems in minimally disordered mixed crystals. Physical Review Letters, 96(23), [235503]. https://doi.org/10.1103/PhysRevLett.96.235503